This depends on your view. These days religion is generally associated seperatly from spirituality. However, the classic definition of religion includes spirituality. Modern usage would consider religion a mass following of worship to a single diety. On the other hand spirituality is more a communion with one's self and nature, which is more focused on the human spirit rather than an exterior spirit.
The question is: Are athiests spiritual? I would imagine some are, some aren't. I don't believe it will go one way or another entirely.