atmosphere in scientific meaning is 大气层、大气、空气圈。
example: 大气污染很严重。=The pollution in atmosphere is extreme.
atmosphere used in daily life with not talking about any scientific things is 气氛、氛围(used for describing the surrounding of people)。
example: 今晚的气氛/氛围真好。 = The atmosphere in here tonight is great.
气氛/氛围 not equal to 大气层、大气
even they are the same word in English