Can I use "sacrilege" as a verb ( Sacrileged ) ?{ to show the robbering of something from a church}

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Look up the verb "to desacrate".  I think this is the word you want.

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Romulus is right. You can say "It is  a sacrilege to steal money from the church".

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I think "sacrilege" is always used as a noun... I'm not sure if "sacrileged" ever exist (and used as a verb).

"sacrilege" is defined as theft of something sacred.

:)